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Although electro-optic (EO) nonlinearities are essential for many quantum and classical photonics applications, a major challenge is inefficient modulation in cryogenic environments. Guided by the connection between phase transitions and nonlinearity, we identify the quantum paraelectric perovskite SrTiO3as a strong cryogenic EO [>500 picometers per volt (pm/V)] and piezo-electric material (>90 picocoulombs per newton) atT= 5 K, at frequencies to at least 1 megahertz. Furthermore, by tuning SrTiO3toward quantum criticality, we more than double the EO and piezo-electric effects, demonstrating a linear Pockels coefficient above 1000 pm/V. Our results probe the link between quantum phase transitions, dielectric susceptibility, and nonlinearity, unlocking opportunities in cryogenic optical and mechanical systems and providing a framework for discovering new nonlinear materials.more » « lessFree, publicly-accessible full text available October 23, 2026
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Tang, Andrew; Audhkhasi, Romil; Saxena, Abhi; Tara, Virat; Ahn, Geun Ho; Vučković, Jelena; Majumdar, Arka (, ACS Photonics)Free, publicly-accessible full text available February 19, 2026
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White, Alexander D; Ahn, Geun Ho; Luhtaru, Richard; Guo, Joel; Morin, Theodore J; Saxena, Abhi; Chang, Lin; Majumdar, Arka; Van_Gasse, Kasper; Bowers, John E; et al (, Nature Photonics)
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Lukin, Daniil M.; Dory, Constantin; Guidry, Melissa A.; Yang, Ki Youl; Mishra, Sattwik Deb; Trivedi, Rahul; Radulaski, Marina; Sun, Shuo; Vercruysse, Dries; Ahn, Geun Ho; et al (, Nature Photonics)
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